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Deeds and legal papers relating to the Crosswood estate, Cardiganshire, 1631, 1705-1820, and to the Plas Llangoedmor estate, 1808-1898, mainly in Cardiganshire and Carmarthenshire.

Deeds and documents of the Williams family of Bodelwyddan, Flintshire, relating to the Bodelwyddan, Bodidris and Pengwern estates in Flintshire and Denbighshire, 1788-1898.

Letters and papers of Rev. John Williams (Ab Ithel) and his family, 1832-1898, comprising page-proofs of parts of Brut y Tywysogion (NLW MS 17163D); drafts and incomplete copies in manuscript of several of Ab Ithel's printed works, including Y Gododdin (NLW MS 17167E), The Traditionary Annals of the Cymry (NLW MS 17168E), Druidism (NLW MS 17169E), Brut y Tywysogion (NLW MS 17164E), and Annales Cambriae (NLW MS 17165E); contributions to the Cambrian Journal (NLW MS 17171E); his address at the Conwy Eisteddfod, 1861 (NLW MS 17187A); papers relating to his collation to the rectory of Llanymawddwy, 1849 (NLW MS 17189E); 'The Church of England independent of the Church of Rome in all ages' (NLW MS 17175B); sermons in English and Welsh (NLW MS 17184C); 'A few plain and practical Observations on Anglican Education' (NLW MS 17185B); the prize essay on the question 'whether the British Druids offered human sacrifices' by 'Hu Gadarn' (NLW MS 17173D); an essay entitled 'Traethawd ar Ddarganfyddiad yr America Gan Madog ab Owain Gwynedd, yn nghylch y ddeuddegfed ganrif' by 'Columbus' (NLW MS 17188C); an essay 'On the state of Agriculture and the progress of Arts & Manufactures in Britain, during the period & under the influence of the Druidical System' by Rev. John Jones, Llanllyfni (see Archaeologia Cambrensis, Supplement 1850) (NLW MS 17176E); 'Y Telynwr Cymreig, sef cyfarwyddiadau i ddysgu'r Delyn' by 'Dafydd Frenin' (NLW MS 17177F); four essays on 'Y manteision a ddeillia i'r Cymry o ddysgu yr iaith Seisnig' by 'Uthr Bendragon', 'Eiddil', 'Gwir Gymro', and 'Y cynyg cynta' 'rioed' (NLW MS 17188C); a 'History of Wales to the death of Llewelyn' (NLW MS 17178E); sections of a work on Christianity in Britain (NLW MS 17179E); letters addressed to Ab Ithel and also to his wife and daughters (NLW MS 17190D); press cuttings and extracts (NLW MS 17181E); sketches and medical and household recipes (NLW MS 17180C), and letters, 1884-1885, relating to the Ab Ithel Memorial Fund.

Deeds and documents, 1515-1898, relating principally to Wales, in particular Cardiganshire, Carmarthenshire, Monmouthshire and Glamorgan. The collection does not relate to a single particular family or estate, but the Cardiganshire documents mainly relate to Aberystwyth and Llanbadarn Fawr.

Holograph letters (26) from W.E. Gladstone, 1841-1897.

Deeds, documents and letters, 1638-1897, relating mainly to properties in Denbighshire and Shropshire, but also Caernarfonshire, Cardiganshire, Montgomeryshire, Merionethshire, Radnorshire and Cheshire; plans relating to the activities of railway companies mainly in the parishes of Gresford and Wrexham, Denbighshire, 1845-1849; and printed material, 1863-1897.

A two-volume collection of pedigrees, mainly of South Wales families, compiled during the 1830s (23967iE watermark 1828; 23967iiE watermark 1831), with some later additions, by David Jones Lewis, Gilfach, Llanwrda, Carmarthenshire.
A duplicate set of these volumes, also written by David Jones Lewis, are the 8 volumes of Gilfach MSS in the College of Arms, London (see Francis Jones, A Catalogue of Welsh Manuscripts in the College of Arms (London, 1988), pp. 69-71), which are dated by colophon to 1830. This duplication is mentioned in a note, dated 8 July 1895, in 23967iE, p. 1, by Lewis's grandson, David Jones Lewis of Llwyncelyn, Llanwrda, who has also overwritten parts of the earlier text, as well as adding pedigrees relating to the Lewis family, [1895] (pp. 1438-50), and a copy of 'an account of the Lewis family in the handwriting of my late grandfather', 1896 (pp. 1494-6). There are minor additions relating to the Lewis family, to at least 1978, in several different hands (pp. 1438-41, 1448-50). A copy of an unpublished account, [1990s], of the Lewis family of Gilfach and Llwyncelyn, including references to the Pedigree Books, is now NLW ex 2511. An index to these two volumes is now NLW MS 23968i-iiE.

Lord Rosebery [Archibald Philip Primrose, 5th earl]: Robert Burns ... (Edinburgh, 1896), being a vellum-bound presentation copy by the author to D. R. Daniel (marked 'For the sake of Tom Ellis ...'), and a covering letter from 'Tom' [Thomas E. Ellis] to David [R. Daniel] which is bound in the volume.

Llawysgrifau Daniel Owen, [1885]-[1895], yn cynnwys drafftiau o'r rhan fwyaf o'i nofel Profedigaethau Enoc Huws (Wrecsam, 1891), a rhannau o'r cyfrolau Y Siswrn (Yr Wyddgrug, 1886), Gwen Tomos (Wrecsam, 1894) a Straeon y Pentan (Wrecsam, 1895). = Manuscripts of Daniel Owen, [1885]-[1895], including drafts of most of his novel Profedigaethau Enoc Huws (Wrexham, 1891), along with parts of the volumes Y Siswrn (Mold, 1886), Gwen Tomos (Wrexham, 1894) and Straeon y Pentan (Wrexham, 1895).

Incomplete typed proof copy of "The Sovereignty of the Bible", [1895], by Morris Owen Evans, PhD, DD, author of 'An essay towards comprehension: Christianity and Churchmanship', 1895, 'The Healing of the Nations', etc.

Manuscripts and printed works, 1818-1895, of Lady Charlotte Guest (née Bertie, other married name Schreiber), comprising journals, 1824-1891 (with gaps); papers relating to the iron and coal industries at Dowlais, 1818-1853; and copies of her printed books, 1888-1895.

Manuscripts of the Rev. Dr Thomas Davies (1833-1899) of Dolgellau, Painswick and London.

A volume containing holograph addresses and poetry in Welsh, 1880-1895, including a copy of a poem composed in 1865 (ff. 118 verso-121 verso) by T. Glwysfryn Hughes; the addresses include 'Daniel O'Connell' (ff. 4-17 verso), 'Goronwy Owen' (ff. 52 verso-68 verso), and 'Ann Griffiths' (ff. 141 verso-160); also included is a transcript, 1883, of minutes relating to the closure in 1865 of Rose Place C. M. Church, Liverpool, and the opening of Fitzclarence Street C. M. Church, Liverpool (f. 2 verso).

Register of members of the Llandyssul Benefit Society, compiled [?1875]-[1895] (watermark 1869), listing members from the establishment of the Society in 1853 to 1895 (ff. 1 verso-30).

Miscellaneous verse and prose in Welsh, [1858]-[1895], by the Rev. T. Glwysfryn Hughes and others, together with a letter, 1884, to Hughes from Robert Parry (Robyn Ddu Eryri) (f. 1).

Manuscripts of D. Griffith Davies, 1887-1894, comprising archaeological notes and heraldic notes and sketches.

A group of poetry and miscellaneous papers from the collection of, and partly in the autograph, of David Griffith (Clwydfardd). They include englynon by Clwydfardd, e.g. 'Ar ymweliad ei rasusolaf Fawrhydi Tywysog Cymru an gwyl Genedlaethol yn Nghaernarfon Gorphenaf [1894]'; 'Ir diweddar barchedig Edward Anwyl Cadeirydd y Dalaith Ogleddol', etc.; englynion addressed to Clwydfardd by Richard Parry (Gwalchmai) and John Cadvan Davies (Cadvan) (1891); copies of the proclamations of meetings of Gorsedd Beirdd Ynys Prydain at national and provincial eisteddfodau; a letter, [c. 1891], from Clwydfardd to B. Morris Lewis, Chelsea, giving particulars of nineteenth century national and other eisteddfodau; notes on the key to 'Coelbren y Beirdd', etc., by T. H. Thomas (Arlunydd Penygarn); incomplete notes on the Epistle to the Hebrews; and an incomplete eulogy of the writing pen, 1872.

Papers of David Richards, 1886-1894, including letters, 1891-1894, to his wife, describing his voyage and stay in the settlement; journal consisting of loose leaves of the journey to Cwm Hyfryd, Patagonia, September 1891 to January 1892; journal of the voyage home from Buenos Aires to Plymouth, July-August 1892; copies of Welsh poems transcribed and possibly composed by David Richards, proofs of, or cuttings containing, parts of a series of articles on 'Cyfoeth Mwnawl y Wladfa Gymreig' to Y Celt in 1891, and a printed copy of a report on the Garn Gold Mine near Dolgellau, 1888.

Scrapbook, 1885-1892, compiled by the amateur actor Augustus Spalding, a close friend and supporter of the opera singer Adelina Patti, containing press cuttings, photographs, printed items, letters and ephemera.
The volume contains material relating to Patti's wedding to Ernesto Nicolini (ff. 11 verso-12 verso, 12c, 13), various charity concerts in Swansea and Brecon (ff. 17-20, 30-31 verso, 41a-b, 42-43, 81-84 verso), her tour of South America in 1888 (in particular Buenos Aires and Montevideo) (ff. 32 verso-36, 39 verso-41 verso), engravings of Craig-y-Nos Castle (ff. 43 verso-45), her birthday party, 19 February 1889 (ff. 50 verso-51), performances at the Patti Theatre, Craig-y-Nos (ff. 62 verso, 67, 78-80 verso, 85), and the Grand Autumn Concert Tour of 1890 (f. 63 recto-verso), all being events in which Spalding participated. The majority of the material however relates to Spalding's acting activities as a member of the Old Stagers during the annual Canterbury Cricket Week, and with the Windsor Strollers.