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Photocopies of sermons, in Welsh, 1869-76, delivered at churches in Bangor and Dwygyfylchi by the Reverend Hugh Davies ('Hywel Ddu o Arfon', d. 1909), who emigrated to Patagonia in 1883 and was a Welsh Chaplain in the Chubut Colony (cf. NLW MS 23383B); and of the diary, 1909-10, of his son Robert Llywelyn Davies (b. 1878), Chubut.

Llungopïau o lythyr W. H. Hughes ('Glan Caeron'), Dolavon, Patagonia, 1925, at Mrs Ellen Jones ('Nel Fach y Books'), Emporium, Llandysul, yn cydymdeimlo â hi ar farwolaeth ei thad, ei 'hen gyfaill' [John Davies] a fu'n byw yn Y Wladfa, ac yn cynnwys newyddion am y datblygiadau yn y wlad a'r twf yn y boblogaeth.

Llungopïau o bedwar llythyr, 1915, oddi wrth aelodau o'r teulu Owen a ymfudodd o Batagonia i Moora, Gorllewin Awstralia, at eu perthynas Maggie Owen yn Abergele. = Photocopies of four letters in Welsh, 1915, from members of the Owen family who emigrated to Moora, Western Australia, from Patagonia, to their relative Maggie Owen in Abergele.

A photocopy of the last letter, 1925, written by 'Glan Caeron' (Guillermo H. Hughes, 1866-1926), Chubut, Patagonia, to his relatives in Wales. = Llungopi o'r llythyr olaf, 1925, a ysgrifennodd 'Glan Caeron' (Guillermo H. Hughes, 1866-1926), Chubut, Patagonia, at ei berthnasau yng Nghymru.

Llungopïau o bapurau'n ymwneud â John Murray Thomas (1847-1924) a ychwanegwyd at y rhai a roddwyd gan Olivia Hughes de Mulhall ym mis Medi 1975; yr oedd John Murray Thomas o Ferthyr Tudful yn wreiddiol ac ymfudodd i'r Wladfa ar y Mimosa gyda'r fintai gyntaf yn 1865. Casglwyd y papurau ynghyd gan Olivia Hughes de Mulhall, gwraig ei ŵyr, tra'n gweithio ar ei llyfr John Murray Thomas: pequeño hombre pero gran héroe para la historia de Chubut (Trelew, 1999), gydag adolygiadau, 2000, ohono. Ymhlith y papurau ceir rhannau o'i ddyddiaduron, 1877, 1878 ac 1893; ei gynllun o Gwm Hyfryd, 1885; ei ohebiaeth, 1888-1911, gan gynnwys deiseb a luniwyd ganddo, 1893, ynglŷn â hawliau tir; pedwar llythyr gwreiddiol at John Murray Thomas, 1895-1898, a chytundeb busnes gwreiddiol, 1893. Ceir papurau hefyd yn ymwneud â'i thad y bardd Morris ap Hughes, gan gynnwys enghreifftiau o'i farddoniaeth fel 'Cerdd ymson wrth feddrod Eluned [Morgan]' a 'Gwyl y Glaniad' mewn Sbaeneg; a chyfieithiadau o emynau adnabyddus Cymreig i'r Sbaeneg gan ei fab Osian Hughes, Eisteddfod Chubut 1988

Papers of and acquired by R. Bryn Williams, mainly relating to the Welsh settlement in Patagonia, including a diary of Joseph Seth Jones, one of the first wave of emigrants on the Mimosa to Patagonia, 1865, and correspondence, 1865-1868; correspondence of his brother, Robert Charles Jones, 1867-1877; copy records of the Welsh courts in Y Wladfa, 1872-1881; letters and minute books relating to Vrondeg Baptist Chapel, 1875-1887, Gaiman, 1877-1891, Eglwys Llanddewi, 1891, Eglwys Bryn Gwyn and Cyfarfod Misol Y Wladfa (Calvinistic Methodists), 1881-1955; papers relating to the Centenary Celebrations of the Welsh settlement in Patagonia, 1952-1962; letters from the founders of the Welsh colony, 1866, and from others who had experienced life there; letters to R. Bryn Williams from Patagonia and from Wales relating to Patagonia, [c. 1941-1961]; research notes and manuscripts of books and radio plays by R. Bryn Williams, 1942-1962; miscellaneous records relating to Wales and elsewhere collected by Williams, 1865-1962; papers relating to John S. Williams, 1901-1962; papers and press cuttings on the history, culture and industry of Patagonia, 1869-1962; and typescripts of published and unpublished works, lectures, scripts, etc.

A collection comprising correspondence, legal papers, press cuttings and other material relating to the Wladfa Gymreig in Patagonia, including material relating to Cwmni Masnachol Camwy; journals of Llwyd ap Iwan and an account by him of the Chubut Valley.

Papers, 1878-1932, of Edward Jones Williams, relating mainly to the Welsh settlement in Patagonia and the Chubut Mercantile Company, comprising preparatory notes relating to the building of the Chubut Railway, c.1907, correspondence relating to both his work and to the Welsh colony, 1909-1932; and printed material, 1909-1932, including annual reports of the Chubut Mercantile Company, 1909-1928.

Papers of John Evans (d.c.1949) of Tre-boeth and Fishguard, Pembrokeshire, including an autobiographical essay,[c. 1949], programmes of eisteddfodau and singing festivals with which he was associated, 1891-1949, manuscript music composed by him, 1893-1948, his eisteddfod adjudications,[c. 1912]-1926, and records and papers relating to his music shop, 1913-1941; papers of his -- daughter Mali Evans d. 1991), including papers, some collected, relating to the Welsh colony in Patagonia and the Welsh diaspora, [c. 1895]-1987, and letters from her uncle, Jack Edwards of Aberystwyth, bookseller, musician and Esperanto enthusiast, 1928-1935, and correspondence of Arthur W. Wade-Evans (1875-1964), Welsh historian, and his daughter Mary Phillips to Mali Evans together with printed articles presented by Arthur W. Wade-Evans to Mali Evans. Four additional items from the printers Lowe & Brydone pertaining to 'Môr o gân yw Cymru i gyd', including receipts and a letter, dated 1928 and 1938, from among the papers of John Evans, were received in March 2019.

Papurau ychwanegol Cymdeithas Cymru-Ariannin, yn cynnwys cynnyrch a beirniadaeth cystadleuaeth rhif 176 yn Eisteddfod Genedlaethol Cymru, Llanelli a'r cylch, 2000, i rai sydd wedi byw yn y Wladfa ar hyd eu hoes, a hefyd deunydd a grewyd ar gyfer 'Cystadleuaeth y Wladfa' yn Eisteddfod Tŷ Ddewi, 2002.

Ffeil o bapurau cystadleuaeth Eisteddfod Genedlaethol y Wladfa, Caerdydd a'r Cylch 2008.

Dwy ffeil o bapurau yn ymwneud a Chymdeithas Cymru-Ariannin, Eisteddfod Genedlaethol Cymru, Meirion a'r Cyffiniau, 2009.

Deunydd o gystadlaethau Cymdeithas Cymru-Ariannin yn yr Eisteddfod Genedlaethol, 1995-2005.

Ffeil o bapurau yn ymwneud a Chystadleuaeth y Wladfa (Rhif 170), Eisteddfod Genedlaethol Cymru, Bro Morgannwg, 2012.

Papers, 1967-1969, mainly comprising travel documents and correspondence, relating to Kyffin Williams's visit to Patagonia. Also included are typescript notes relating to Patagonia, [?1961x1962], belonging to John Ormond and used by him in preparation for his visit to the region to film 'The desert and the dream' (1962). These notes, which include an annotated script of the film, appear to have been given to Kyffin Williams, together with a holograph poem by John Ormond, 'Instruction to settlers', 1967, prior to his trip. In addition, the file includes a copy of the journal Argentina, vol. 4, no. 4 (April 1963), which contains an article entitled 'The desert and the dream'; a list of contacts in Patagonia, [1968], prepared by Valmai Jones in readiness for Kyffin Williams's visit; typescript questions and answers prepared before, or possibly at the beginning of, his visit; and a catalogue of the 'Photographs of Patagonia' exhibition at Oriel Môn, 1982, with photocopies of drawings contained in an album. The file also contains a photocopy of the book Tan tro nesaf by Gareth Alban Davies (Llandysul, 1976), which includes the titles of pictures by Kyffin Williams to be inserted in the work.