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A note in the autograph of Thomas Telford, engineer, at London, of 'Improvements necessary to be Undertaken' to the Holyhead Road, together with an estimate of the cost, 26 March, 1822 (references to portions of the road west of Bettws y Coed, between Cerig y druidion and Glyndyffws, between Glyn Dyffws and the Druid, between Corwen and Owen Glyndwrs Hill, and between Rhysgog and Llangollen); and a holograph letter from James Watt, engineer, London, to Robt. Muirheid, Glasgow, 1814 (advice in connection with a voyage along the Welsh coast, from Amlwch to the Bristol Channel).

Four autograph letters, 1764-1784, from Selina, Countess of Huntingdon to Charles Wesley, Thomas Newton (Bishop of Bristol) and 'The Revd Mr. Green' (Norwich), the last being written from her college at Trevecka.

Papers, lecture and research notes of and acquired by Mary Williams, relating to Middle French, Middle Welsh and medieval literature and Arthurian studies, 1907-1963; books collected by Mary Williams, 1897-1911; letters to Prof. Victor Spiers, 1898-1916; vouchers and receipts, 1924-1973; newspaper cuttings, 1911-1940; school books 1909-1916; papers relating to University College Swansea, 1921-1975, University of Wales Aberystwyth, 1924-1974, University of Durham, 1948-1952, and National Library of Wales, 1941-1974; correspondence, 1927-1976; and family papers, 1898-1944.

A manuscript copy, [1820s]-[1830s] (watermark 1814), of tours of North Wales undertaken in the Autumn of 1817 (pp. 1-30) and October 1819 (pp. 31-90) by Captain Henry Hanmer and his wife Sarah, including descriptions of visits to Lady Eleanor Butler and Sarah Ponsonby, the Ladies of Llangollen (pp. 10-11, 14-19, 45).
The itinerary includes Llangollen, Wrexham, Beddgelert, Caernarfon, Bangor, Llanberis, Holyhead, Conway and St Asaph, and includes descriptions of Dolbadarn Castle (pp. 55-58), the Penrhyn slate quarries (pp. 65-66) and Parys and Mona copper mines (pp. 69-73). A number of related poems and tales are interspersed throughout the text (pp. 4-101), including verses by Anne Grant (p. 19), Anna Seward (pp. 22-29), Sir Walter Scott (pp. 31-33), W. Sotheby (pp. 37-45), W. R. Spencer (pp. 48-53), Dr [William] Dodd (pp. 61-62), and Amelia Alderson Opie (pp. 88-89). They are followed by further transcripts in the same hand (pp. 107-120), including verses by Thomas Noel (pp. 112-118) and Sir Walter Scott (pp. 119-120), and, in a different hand (pp. 121-139), verses by Byron (pp. 121, 125), R. B. Sheridan (p. 121) and Robert Southey (p. 123). The volume contains numerous cuttings from engravings, either pasted or tipped in (pp. 1-103 passim); several of these are by Henry Gastineau and are taken from Wales Illustrated: In a Series of Views... (London, 1830), as is the printed description of Llangollen on pp. 101-102. Inserted at the end (pp. 187-198) is a pamphlet by S. G. Perceval, The Ladies of Llangollen: New and interesting facts ([?1909]), transcribing extracts from the present manuscript. A press cutting, [1829], concerning the Ladies of Llangollen is pasted inside the front cover. Pressed flowers are pasted in on pp. 57, 64-65, and the remains of a leaf has been placed in an archival envelope.

A notebook, [2]-[10] August 1826 (watermark 1824), by the artist the Rev. John Parker of Sweeney Hall, containing the concluding part of an account of a tour to Killarney, Ireland, being a continuation of his journal, now NLW MS 18248A.
Parker describes excursions in the area of Killarney and its lakes (ff. 1-9 verso), including visits to the island of Innisfallen (ff. 2 verso-4, 5 recto-verso), and to Aghadoe (ff. 4-5), followed by the return journey to Britain via Cork (ff. 10 verso-12), Cashel (ff. 12 verso-16), and Dublin. There are frequent descriptions of scenery and of architectural features, including a lengthy description of the Rock of Cashel (ff. 13-15), and there are references throughout to sketches drawn by him. A letter delivered by Parker in Killarney from a 'Miss Ponsonby' is probably from Sarah Ponsonby, one of the Ladies of Llangollen (f. 8 verso). The 'Mr O'Connell and his brother (not the counsellor)' referred to on ff. 2 recto-verso are probably the two younger brothers of Daniel O'Connell. The text includes a poem in praise of Killarney by the author (ff. 3-4).

A photostat facsimile of a priced copy of the catalogue of the contents of Plas Newydd, the residence of the 'Ladies of Llangollen', sold by auction the week beginning 13 August 1832.

A volume, 1863, entitled Letters from Llangollen and based on a series of nineteen letters describing a tour in North Wales and which were published in the Sheffield Daily Telegraph in September 1863. Cuttings from the paper are interspersed with illustrative prints (mainly of churches, castles and other edifices in Wales and England), a few cuttings from other sources, and additional manuscript notes apparently by the author, John Holland.
There are references to the 'Ladies of Llangollen' (ff. 19-22), Dinas Brân (ff. 23-25 verso) and other local features of Llangollen. Pasted onto f. 38 is an envelope, postmarked at Sheffield, 12 September 1863, and addressed to John Holland at Upper Bangor, together with a photograph presumably originally enclosed in the envelope and which probably depicts Holland's correspondent.

Over seventy letters, [c. 1799]-1832, mainly from Lady Eleanor Butler and Miss Sarah Ponsonby, The Ladies of Llangollen (ff. 1-118 verso), addressed to their friend, Mrs Margaret Wingfield (1778-1835) and her husband, the Reverend Rowland Wingfield, vicar of Rhiwabon. The letters contain personal and local news.

A manuscript containing notes made on reading Joseph Butler, The Analogy of Religion or the Welsh translation of it by John Hughes (1827-1893), published at Denbigh in 1859; an essay entitled Elfenau Dedwyddwch a Llwyddiant Teuluaidd, with an English version; translations of historical and religious works; etc.

Papers of the Breton nationalist Louis Feutren (1922-2009), together with papers of two fellow nationalists accumulated by him, Neven Henaff (Célestin Lainé, 1908-1983), and Alan Heusaff (1921-1999). All three were prominent members of the Breton collaborationist force 'Bezen Perrot' formed in December 1943, and all three eventually fled to Ireland sometime after the Second World War. Some of the papers relate to the activities of 'Bezen Perrot', but most are later personal papers.

Proof-sheets of an article by Professor Mary Williams, Swansea (1882-1977) entitled The Dying God in Welsh Literature, with manuscript corrections by the author.

A short biographical sketch of Dr Mary Williams (1883-1977), linguist and former Professor of Modern Languages, University College, Swansea, written by the donor's mother shortly after the subject's death in October 1977.

A small collection consisting of a notebook and legal and other papers of George Stephens, governor of the county gaol, Carmarthen; journals of William Davies, Pumpsaint, midshipman; and a play by George Arbour Stephens entitled 'Carmarthen. A Historical Episode ...'.

Swansea Council Year Book, 1935, with manuscript entries by Dr. G. Arbour Stephens, Swansea, relating largely to his world cruise.

Holograph and/or typescript copies of addresses by George Arbour Stephens, M.D., Swansea, including 'Was Dozmare Pool a Celtic lake of the Underworld?', published in Folk Lore, March, 1935, 'A Green Cross Service for the Celtic Fringe', delivered at the Celtic Congress, Isle of Man, 4 July, 1935, 'The Topographical Importance of Kidwelly and the Burry Estuary in connection with the Arthurian Romances. Caerwen as the old name for Kidwelly', published in The Carmarthen Journal, 25 November, 1938, and 'Radnorshire as a Centre of Celtic Mythology', delivered to the Radnorshire Antiquarian Society at Llandrindod, 2 December, 1938; together with some miscellaneous papers of G. Arbour Stephens, including army certificates, 1897-1918, notices of the leet court with view of frank-pledge of the borough and manor of Swansea, 1919-31, etc.

Deeds, 1542-1797, relating to properties in Glamorgan, Brecknockshire and Carmarthenshire; memorandum book of ?Samuel Owsley and William Owsley of Brecon, with notes on rents, taxes and local events and history, 1679-1768; fragment of an antiphonal, [15th century]; a copy of The Reports of Sir Henry Hobart, Lord Chief Justice of Common Pleas, 1650; and a copy of The Larvae of the British Lepidoptera and their food plants, 1880.

Photocopies from the catalogue of the manuscripts of R. Gwyneddon Davies held at the University of Wales Bangor compiled by his son R[obert] G[wyneddon] D[avies], 1916-1917.

Transcripts, extracts, and notes, [c. 1921], by E. Alfred Jones, M.A., F.S.A., London, relating to the formation and development of Volunteer Companies in Wales during the late eighteenth and early nineteenth centuries, including Caernarvon and Bangor Volunteer Infantry, Loyal Newborough Volunteer Infantry, Snowdon Rangers Riflemen Volunteer Infantry, Conway Volunteers, Loyal Eifionydd Volunteer Infantry, Royal Welch Volunteers, Swansea Gentlemen Volunteer Yeomanry Cavalry, Pembrokeshire Yeomanry Cavalry, etc. (see also NLW MS 11557D).
Among the papers are holograph letters, 1921 and undated, from C. E. Breese, Portmadoc; Hugh Edwardes, 6th baron Kensington; R. L. Harmsworth [1st bart.], London; J. E. Jones, Rhosygwaliau Vicarage, Bala; Ll. Wynne Jones, The Deanery, St. Asaph; Lloyd Tyrell-Kenyon, 4th baron Kenyon; John T. D. Llewelyn [1st bart., of Penlle'r-gaer]; Llewelyn Nevill Vaughan Mostyn, 3rd baron Mostyn; Walter FitzUryan Rhys, 7th baron Dynevor; E. C. Stevens, Wynnstay, Ruabon, for Sir [Herbert Lloyd] Watkin Williams-Wynn, 7th bart.; Bertha Turnorm, for her niece, Joan Emily Mary Campbell, Countess Cawdor; Ernest Edmund Henry Malet Vaughan, 7th earl of Lisburne; Griffith Williams, the Rectory, Llanrwst; Fred[erick] G. Wynn, Glynllivon, Llanwnda; and T. A. Wynne Edwards, Plas Nantglyn, Denbigh.

An order, signed by Charles Williams Wynn (1775-1850), to pay £13.3.6 to the Governor and Company of Chelsea Waterworks for supplying water to the Treasury and to other houses and stables belonging thereunto from 10 October 1805 to 5 January 1806.

This collection comprises poetry by Robert Southey and correspondence between him and his friend and patron Charles Watkin Williams Wynn, son of Sir Watkin Williams Wynn, 4th bart, of Wynnstay, Denbighshire, also letters to Charles's brother, Sir Henry Watkin Williams Wynn. There are 540 letters from Southey to Charles, 364 from Charles to Southey and 759 from Charles to Henry (see also NLW MSS 2789-2806).