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Records relating to the Brigstocke family, including deeds of properties in Carmarthenshire and Pembrokeshire prior their acquisition by the Brigstockes, 1496-1889; deeds and documents of members of the Brigstocke family, 1655-1912; miscellaneous deeds, documents and papers relating to the Brigstocke family and lands in Carmarthenshire, including the Dolhaidd estate, 1846-1892, Cenarth, 1741-1838, and Llandyfaelog and Kidwelly, 1772-1833; legal papers, 1751-1775; and deeds and documents collected by W. Evans George relating to other estates, including: papers of the Lewes family of Gellidywyll, mostly bills and receipts, 1741-1792; draft deeds of W. Evans George for property in the Lower Teifi Valley, Cardiganshire and Carmarthenshire, 1896-1922; sale and account books of W. Evans George and Sons, 1863-1884; printed material, 1837-1925; papers concerned with local elections in Cardiganshire, 1741-1937; weekly account book of the surveyor of the South Wales Highway for Llanfihangel-ar-arth, 1866-1873; records of the Court of Petty Sessions, Penrhiw-pal, Cardiganshire, 1903-1927; and records of the Newcastle Emlyn Town Improvement Committee, 1903-1906.

The series comprises small notebooks which Condry carried with him, recording descriptions of places visited, observations on wildlife, particularly birds and plants, geology, industry, historical landmarks, archaeology, personal reminders, ideas for writing and lecturing, photography, bibliographies, useful contacts and conservation issues, 1952-1994. The main geographical areas covered are Bardsey Island, Cader Idris, Cardiganshire and Merionethshire. An index to the series is provided., compiled by Ceridwen Lloyd-Morgan, 2013.

The papers consist of the personal papers and letters of, and acquired by, Evan Richards of Nanthenfoel, 1823-1872; family correspondence, 1826-1891; unproved Cardiganshire wills, 1805-1847; and miscellaneous documents of Cardiganshire interest, 1787-1853.

A manuscript in the hand of J. H. Davies recounting the activities of Lewis Morris ('Llywelyn Ddu o Fôn') in Cardiganshire (with particular reference to the incidents at Esgair-mwyn lead mine in 1751-3 which led to his imprisonment); and a typescript article by [J. H. Davies] entitled 'Morysiaid Môn a'u lle yn Hanes Cymru'.

Correspondence and papers of T.G.G. Herbert together with historical records acquired by him, 1736-1899, general and political correspondence, 1953-1986, much of it relating to the work of the Ceredigion District Council; papers relating to the Cardiganshire County Council elections, 1955-1972; personal papers, 1936-1988; and papers relating to his son Rhodri Herbert, 1954-1972.

An additional five boxes of papers were donated February 2006. This group remains uncatalogued. A collection of photographs, slides and postcards were received at the same time, which also remain uncatalogued.

Papers of Tom Owen, HMI, of Aberystwyth, Cardiganshire, 1898-1966, mainly relating to his career in education, including inspector's reports on schools in Montgomeryshire, 1946-1950; reports on St. David's College, Lampeter, Cardiganshire, 1907-1945; and personal papers, 1898-1966.

Papers, 1839-1971, relating to farming in Cardiganshire, including agricultural notebooks, 1839-1919, accounts for payments to servants, 1879-1894, accounts of live and dead stock, 1879-1887; business letters, 1890-1918, letters to Richard Phillips, 1890-1901; personal letters, 1868-1971; literary material, late 19th cent.-1940; domestic accounts, 1898-1930; diaries, 1898-1954; papers relating to Tabor Calvinistic Methodist Chapel, Llangwyryfon, 1860-1926; and to Talybont school, and Llanilar parish council papers, 1892-1899.

Records of the Cardiganshire Liberal Association, 1921-1974, including minute books, 1923-1951; correspondence, financial and other papers, 1914-1974; electoral registers, 1951-1964; press cuttings of political interest, 1900-1963.

A certificate of the admission and enrolment, on 3 March 1814, of the Reverend Thomas Edwards, clerk, minister of Llanddeiniol, as a burgess of the town and liberties of Cardigan; press cuttings, including copies of articles entitled 'Reminiscences of Mid-Cardiganshire' contributed by Evan Edwardes to The Welsh Gazette, 1908.

Deeds, 1555-1918, of clients and relating to properties in Cardiganshire, Merionethshire, Montgomeryshire and Radnorshire, including papers of the Penglais estate in the Aberystwyth area, 1555-1918; Aberystwyth borough records, 1759-1813; letters, 1794-1882; papers of John Parry, solicitors, Aberystwyth, including share certificates of the Aberystwyth Gas and Coke Company, 1839; Bwlch Consolidated Lead Mines, 1847; records concerning the Aberystwyth and Tregaron Bank, 1813-1844; miscellaneous papers, [c. 1783]-1932; printed items, [c. 1783]-1867; certificates of shares in the Aberystwyth Public Rooms, 1818-1821, and the Robinson Gold Mining Company, 1903; letters and papers relating to the estate of Roderick Richards, Penglais, [c. 1830]; builders' accounts, 1845; and tithe receipts, 1927-1932.

Miscellaneous papers, 1920-1923, concerning various aspects of life in Cardiganshire.

Papers, 1907-1988, mainly relating to the activities of the Labour Party in Carmarthenshire and Cardiganshire, 1917-1967, including: papers of the Llanelli Trades Council and Divisional Labour Party, including minute books, 1940-1967; accounts, financial papers and cash books, 1925-1967; correspondence, 1921-1967; miscellaneous papers, 1917-1967; press cuttings, 1926-1959; and general election papers, 1931-1964; political and professional papers of Loti Rees Hughes, including correspondence, minute books and press cuttings, 1927-1965; and personal and family papers, 1935-1969; papers of W. Douglas Hughes [c. 1920]-1968, including correspondence, 1932-1967; notebooks, c. [1920]-1966; and correspondence and papers relating to Carmarthenshire County Council, 1944-1968; together with the papers of Dr Deian R. Hopkin, 1907-2000, including correspondence, 1962-2000; and miscellaneous printed material, with some concerning the Labour Party, 1907-1984 and the University College of Wales, Aberystwyth, 1960-1973.

An album containing press cuttings, reprints of articles in the Aberystwyth Observer, 1899-1905, posters, etc., mainly relating to Aberystwyth and Cardiganshire, and minutes of the committee of the 'Highgate Men's Club', Whitchurch, Shropshire, founded in 1889, with correspondence and other papers relating to the club.