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Deeds relating to the Pit, Dorstone, Herefordshire, and to Brook House, Llanigon, Brecknockshire, 1754-1965; and deeds relating to a cottage in Llanigon, 1854-1898.

Records of the Broom Hall estate, Caernarfonshire, 1625-1939, comprising deeds, 1567-1946, rent books and rentals, 1787-1816, 1856-1942, ledgers, 1907-1937, cash books, 1907-1939, wages books, 1905-1946, and correspondence, 1748-1925, deeds, 1664-1808, and account and rent books, 1785-1871, of properties in St James Westminster and St Martin in the Fields, Middlesex; deeds relating to the Bodfel estate, Caernarfonshire, 1725-1854; rentals of the Madryn estate, 1816-1819, and Meillionydd estate, 1846-1857, both in Caernarfonshire; and a record of the average price of corn, 1771-1826.

Documents, mostly acquittances for legacies bequeathed by William Lloyd of Conwyl Gaeo, gent., 1787, deeds relating to properties in the parishes of Caeo, Llanycrwys and Talley, Carmarthenshire, and Lledrod, Cardiganshire,1776-1870, and accounts, mainly of the Brunant estate in the parish of Caeo, 1856-1886.

Deeds and documents, 1591-1901, relating to properties in the Llanfyllin area, Montgomeryshire, and in Shropshire.

Papers, [1950]-[1999], relating to Bryn Owen's research on the history of the Welsh militia.

Deeds, 1564-1857, relating to the Bachegraig estate, Flintshire; brief diary entries of Gabriel and Hester Lynch Piozzi, 1797-1812 (NLW MSS 11096-102); correspondence, 1756-1823 (NLW MS 11103D); heraldic and genealogical records, 1813 (NLW Rolls 223); and a survey and valuation of the Bachegraig estate, 1790, which also includes accounts, 1788-1807 (NLW MS 11104C).

Deeds and documents relating to the Mostyn family of Bryngwyn, Montgomeryshire, and Plas Kynaston, Denbighshire, 1729-84, and their successors, the Owen family of Woodhouse, Shropshire, 1774-1813.

Papers of Brynmor T. John, 1970-1988, mainly relating to his career as a politician, including Constituency and Parliamentary correspondence and papers, 1970-1985; Constituency correspondence and papers, 1986-1988; records relating to the Pontypridd Division Labour Party, 1919-1970; records relating to the Labour Party, 1967-1976; papers relating to local government, 1967-1989; papers relating to general elections, 1966-1987; and papers relating to foreign affairs, 1965-1973.

Papers of Brythonydd and others, [early 18th century]-1952, comprising essays and notes on Teifiside history, 1902-1909; notes on sermons and lectures; diaries, 1906-1923; transcripts of various historical, literary and religious material including Ystradyfodwg parish records, 1735-1930, and Howel Harris' diaries, 1738-1771; transcripts of poetry by Cardiganshire poets including Gwinionydd; letters, 1898-1952; vestry books and account books of Cenarth and Penbryn and other parishes, [pre 1798]-1876; records of Libanus, Treherbert including minute books, registers and account books, 1842-1946; papers of Benjamin Williams (Gwinionydd), including letters, sermons, 1855-1890, essays, notes and poetry; papers of David James (Defynnog), Treherbert, relating mainly to the column he edited in The South Wales News and including sermons and adjudications of his uncle, Benjamin Thomas (Myfyr Emlyn), 1875-1928; papers of John Morris Jones (Ioan Cunllo), John Thomas, Charles Davies, Thomas Cynfelyn Benjamin, Lewis Jones, Treherbert, Rees Price, David Price, Joseph Davies and Rhys Lloyd Jones, Troed-yr-aur, and others, consisting mainly of poetry, accounts, letters, addresses, notebooks and sermons, [19th century]-[20th century].

Papers of the Waddington, Bunsen and Chisholm families, consisting mainly of letters to Mrs Georgina Waddington of Llanover from her eldest surviving daughter, Frances, and her husband Christopher Charles Bunsen, 1817-1825, mainly written from Rome where Bunsen was Charge d'Affairs; letters to Thomas Waddington mainly from his his wife Janet Waddington (nee Chisholm), 1825-1866; letters to Janet Waddington, [c.1825]-1845, from members of the family; letters to Catherine Chisholm, 1826-1843, mainly from Janette Waddington; letters to Mrs Eliza Chisholm, 1825-1845; and letters to Frances Chisholm, 1822-1841.

Deeds, mostly relating to the estate of the Burchinshaw family, Denbighshire, 1668-1750, and the Tremadog, Caernarfonshire, estate of the Roche family, 1895-1900.

Family papers and estate records of the Burchinshaw family of Llansannan, Denbighshire, 1557-1863.

Deeds and documents, 1719-1855, relating mainly to the Peniarth estate in Merionethshire and Caernarfonshire, mainly leases, bonds and mortgages, 1728-1767.

This collection comprises account books relating to the erection of the Welsh Calvinistic Chapel at Cwmystwyth, Cardiganshire, 1836; correspondence and papers, 1886-1900, relating to The Cambro-Briton Society, London and to some other aspects of the London Welsh community; material relating to the Welsh Hospital for South Africa, to the National Eisteddfod held in London, 1887, and to preaching activities in Croydon, Enfield, Harrow and Willesden.

Records mainly of the Glamorgan estate of the marquesses of Bute and of their predecessors, the earls of Pembroke. These include letters, 1588-1855, including letters of the Herbert family of Cogan Pill, 1588-1719, but primarily the personal and estate correspondence of John, second marquis of Bute, 1804-1855, (including letters relating to Bedfordshire, Cambridgeshire (Kirtling: Lady Bute's property) and County Durham estates); deeds, [1319]-1937; surveys, 1570-1842; rentals of the Glamorgan estate, 1728-1893, and the Cardiff estate, 1842-1895, estate and manorial accounts, 1573-1873; manorial records and deeds of over seventy manors, mainly in Glamorgan, [?1373]-1847; family settlements, [early 17 cent.]-1902; family probate records, 1612-1900; and legal and case papers, 1642-1921; correspondence of Alice, Lady Windsor, 1757-1776; a substantial number of copies of Acts of Parliament, relating mainly to roads, canals, docks and harbours, railways, public works and utilities, 1771-1928; and miscellaneous records. -- The archive illustrates the history of Glamorgan; the corporate life of the boroughs of Cardiff, Cowbridge and Llantrisant; the urbanization of the South Wales valleys, especially Merthyr Tydfil and Aberdare; the Glamorgan Commission of the Peace; the county militia and yeomanry, 1815-1837; the development of the coal and other industries (it includes papers relating to minerals and ironworks 16th-early 20th cent., accounts of coal shipped from Neath, etc. 1626-1682, quarry and lime kiln accounts 19th cent. Cardiff railway, dock and harbour papers and plans, 19th-20th cent.); labour and political unrest, including Chartism, Scotch Cattle, Rebecca riots; early trade unions; and the history of Cardiff castle, 16th-19th cent., including inventories 1581, 1585, estimate of repairs 1590 and plans of grounds.

Deeds, 1629-1833, relating to the families of Lucas and Matthews of Bwlch-hafod-y-gof, Llangurig, Montgomeryshire.

Sales ledgers, 1891-1930, 1940-1944, and 1949-1958, and purchase ledgers, 1894-1925.

Planning documents and reports relating to four-year development plans: Sixth Plan, 1971-1975; Seventh Plan, 1976-1980; Eighth Plan, 1980-1984; reports on administration of the Loire, Brittany and Ile et Vilaine region, 1974-1979; minutes of C E S and sub-committees, 1974-1979; miscellaneous pamphlets and publicity material on nuclear power, 1974-1979; printed and official reports, 1971-1980; correspondence and related papers of the Amoco Cadiz disaster, 1978-1979, the 'Plan medico-hospitalier breton', 1973-1975, and protests by medical students at Rennes, 1973, C E L I B (Comite d'etude et de liaison des interets bretons) [Breton studies committee]), 1972-1978, the Institut Culturel Breton, 1972-1979; the Charte Culturelle de Bretagne, 1975-1979; the Conseil Culturel de Bretagne, 1978-1979; and 'L'annee du patrimoine', 1979-1980.

Deeds, 1591-1857, relating to land in the parishes of Pennard, Llangyfelach, Wick, St. Johns (Neath), Neath, Bishopston, Llangiwg, Penrice, and Swansea, all in the county of Glamorgan; estreats, 1747-1800, of the manor of Ogmore, Glamorgan.

C. L. J. Humphreys family papers some of which relate to Charles Jones Humphreys, Charles Milward Dovaston Humphreys and Charles Humphreys, comprising family correspondence, probate and related papers, deeds, papers relating to the Pennant estate, [Montgomeryshire], together with genealogical papers, 1712-1958; and the C. L. J. Humphreys deeds and documents comprising twenty-four deeds, 1647-1802, relating to the Thomas and Humphreys families of Pennant concerning properties in the parishes of Betws, Berriew, Llandyssil, Llanmerewig, Newtown and Llanllwchaearn, Montgomeryshire, together with a plan, 1763, relating to the property of Charles Humphreys in the parish of Llandyssil.